We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Néel temperature TN∼77K pointed out by a huge Debye-Waller σ2 factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T∗=150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.

Castellano, C., Berti, G., Sanna, S., Ruiz Bustos, R., Van Duijn, J., Brambilla, A., et al. (2015). Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7. PHYSICAL REVIEW. B, CONDENSED MATTER AND MATERIALS PHYSICS, 91(22), 1-6 [10.1103/PhysRevB.91.224101].

Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7

SANNA, SAMUELE;
2015

Abstract

We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Néel temperature TN∼77K pointed out by a huge Debye-Waller σ2 factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T∗=150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.
2015
Castellano, C., Berti, G., Sanna, S., Ruiz Bustos, R., Van Duijn, J., Brambilla, A., et al. (2015). Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7. PHYSICAL REVIEW. B, CONDENSED MATTER AND MATERIALS PHYSICS, 91(22), 1-6 [10.1103/PhysRevB.91.224101].
Castellano, C; Berti, G.; Sanna, Samuele; Ruiz Bustos, R.; Van Duijn, J.; Brambilla, A.; Muñoz Noval, Á.; Carretta, P.; Duò, L.; Demartin, F....espandi
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Utilizza questo identificativo per citare o creare un link a questo documento: https://hdl.handle.net/11585/554690
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