We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Néel temperature TN∼77K pointed out by a huge Debye-Waller σ2 factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T∗=150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.
Castellano, C., Berti, G., Sanna, S., Ruiz Bustos, R., Van Duijn, J., Brambilla, A., et al. (2015). Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7. PHYSICAL REVIEW. B, CONDENSED MATTER AND MATERIALS PHYSICS, 91(22), 1-6 [10.1103/PhysRevB.91.224101].
Evidence of local structural order and spin-lattice coupling in the frustrated pyrochlore Y2Ru2 O7
SANNA, SAMUELE;
2015
Abstract
We present an extended x-ray absorption fine structure study of the pyrochlore Y2Ru2O7 (8-298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the Néel temperature TN∼77K pointed out by a huge Debye-Waller σ2 factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at T∗=150 K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.