Analytic expressions of the direct, resonant and interference contributions to the differential cross section of a resonant Auger process, produced by the photoionization of a linear molecule either "fixed-in-space" or belonging to a gas of randomly oriented molecules, have been derived following Dill's procedures but going beyond the two-step approximation. Angle-resolved Auger spectra of the C2H2 molecule measured on top of the C1s->pi* resonance have been calculated and compared with experiments, analysing also the different contributions to the electron angular distributions.
R.Colle, D.Embriaco, M.Massini, S.Simonucci, S.Taioli (2004). Ab initio calculation of angle-resolved resonant Auger spectra of C2H2. RENNES : K.M.Dunseath and M.Terao-Dunseath.
Ab initio calculation of angle-resolved resonant Auger spectra of C2H2
COLLE, RENATO;
2004
Abstract
Analytic expressions of the direct, resonant and interference contributions to the differential cross section of a resonant Auger process, produced by the photoionization of a linear molecule either "fixed-in-space" or belonging to a gas of randomly oriented molecules, have been derived following Dill's procedures but going beyond the two-step approximation. Angle-resolved Auger spectra of the C2H2 molecule measured on top of the C1s->pi* resonance have been calculated and compared with experiments, analysing also the different contributions to the electron angular distributions.I documenti in IRIS sono protetti da copyright e tutti i diritti sono riservati, salvo diversa indicazione.
